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Surface modification of biomaterials by photochemical immobilization and photograft polymerization to

Yakai FENG, Haiyang ZHAO, Li ZHANG, Jintang GUO,

《化学科学与工程前沿（英文）》 2010年 第4卷 第3期   页码 372-381 doi: 10.1007/s11705-010-0005-z

摘要： Thrombus formation and blood coagulation are serious problems associated with blood contacting products, such as catheters, vascular grafts, artificial hearts, and heart valves. Recent progresses and strategies to improve the hemocompatibility of biomaterials by surface modification using photochemical immobilization and photograft polymerization are reviewed in this paper. Three approaches to modify biomaterial surfaces for improving the hemocompatibility, i.e., bioinert surfaces, immobilization of anticoagulative substances and biomimetic surfaces, are introduced. The biomimetic amphiphilic phosphorylcholine and Arg-Gly-Asp (RGD) sequence are the most effective and most often employed biomolecules and peptide sequence for improving hemocompatibility of material surfaces. The RGD sequence can enhance adhesion and growth of endothelial cells (ECs) on material surfaces and increase the retention of ECs under flow shear stress conditions. This surface modification is a promising strategy for biomaterials especially for cardiovascular grafts and functional tissue engineered blood vessels.

关键词： biomimetic amphiphilic     amphiphilic phosphorylcholine     endothelial     functional     biomaterial    

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Identification of sources, characteristics and photochemical transformations of dissolved organic matter

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1340-z

摘要：

• The source of DOM in surface water and sediment is inconsistent.

关键词： Dissolved organic matter     Parallel factor analysis     Excitation-emission matrices     Photodegradation    

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Peroxyacetyl nitrate measurements by thermal dissociation–chemical ionization mass spectrometry in an urban environment: performance and characterizations

Xinfeng Wang, Tao Wang, Likun Xue, Wei Nie, Zheng Xu, Steven C. N. Poon, Wenxing Wang

《环境科学与工程前沿（英文）》 2017年 第11卷 第4期 doi: 10.1007/s11783-017-0925-7

摘要： Peroxyacetyl nitrate (PAN) is an important indicator of photochemical smog and has adverse effects on human health and vegetation growth. A rapid and highly selective technique of thermal dissociation–chemical ionization mass spectrometry (TD-CIMS) was recently developed to measure the abundance of PAN in real time; however, it may be subject to artifact in the presence of nitric oxide (NO). In this study, we tested the interference of the PAN signal induced by NO, evaluated the performance of TD-CIMS in an urban environment, and investigated the concentration and formation of PAN in urban Hong Kong. NO caused a significant underestimation of the PAN signal in TD-CIMS, with the underestimation increasing sharply with NO concentration and decreasing slightly with PAN abundance. A formula was derived to link the loss of PAN signal with the concentrations of NO and PAN, which can be used for data correction in PAN measurements. The corrected PAN data from TD-CIMS were consistent with those from the commonly used gas chromatography with electron capture detection, which confirms the utility of TD-CIMS in an urban environment in which NO is abundant. In autumn of 2010, the hourly average PAN mixing ratio varied from 0.06 ppbv to 5.17 ppbv, indicating the occurrence of photochemical pollution in urban Hong Kong. The formation efficiency of PAN during pollution episodes was as high as 3.9 to 5.9 ppbv per 100 ppbv ozone. PAN levels showed a near-linear increase with NO concentration, suggesting a control policy of NO reduction for PAN pollution.

关键词： TD-CIMS     Peroxyacetyl nitrate     Interference     Photochemical pollution     Formation efficiency    

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Photochemical indicators of ozone sensitivity: application in the Pearl River Delta, China

Lyumeng Ye,Xuemei Wang,Shaofeng Fan,Weihua Chen,Ming Chang,Shengzhen Zhou,Zhiyong Wu,Qi Fan

《环境科学与工程前沿（英文）》 2016年 第10卷 第6期 doi: 10.1007/s11783-016-0887-1

摘要： The distribution of NO - and VOC-sensitive regimes in the PRD are identified. The effectiveness of six popular chemical indicators for discriminating O sensitivity regimes is evaluated. Threshold levels for HCHO/NO , H O /HNO , O /NO , O /NO , O /HNO were derived and verified. The indicators H O /HNO and H O /NO performed best and maintained relatively stable threshold levels. Surface O production has a highly nonlinear relationship with its precursors. The spatial and temporal heterogeneity of O -NO -VOC-sensitivity regimes complicates the control- decision making. In this paper, the indicator method was used to establish the relationship between O sensitivity and assessment indicators. Six popular ratios indicating ozone-precursor sensitivity, HCHO/NO , H O /HNO , O /NO , O /NO , O /HNO , and H O /NO , were evaluated based on the distribution of NO - and VOC-sensitive regimes. WRF-Chem was used to study a serious ozone episode in fall over the Pearl River Delta (PRD). It was found that the south-west of the PRD is characterized by a VOC-sensitive regime, while its north-east is NO -sensitive, with a sharp transition area between the two regimes. All indicators produced good representations of the elevated ozone hours in the episode on 6 November 2009, with H O /HNO being the best indicator. The threshold sensitivity levels for HCHO/NO , H O /HNO , O /NO , O /NO , O /HNO , and H O /NO were estimated to be 0.41, 0.55, 10.2, 14.0, 19.1, and 0.38, respectively. Threshold intervals for the indicators H O /HNO , O /NO , O /NO , O /HNO , and H O /NO were able to identify more than 95% of VOC- and NO -sensitive grids. The ozone episode on 16 November 16 2008 was used to independently verify the results, and it was found that only H O /HNO and H O /NO were able to differentiate the ozone sensitivity regime well. Hence, these two ratios are suggested as the most appropriate indicators for identifying fall ozone sensitivity in the PRD. Since the species used for indicators have seasonal variation, the utility of those indicators for other seasons should be investigated in the future work.

关键词： Ozone     Pearl River Delta (PRD)     Sensitivity regime     Photochemical indicator     Threshold levels    

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Atmospheric heterogeneous reaction of chlorobenzene on mineral -FeO particulates: a chamber experiment study

《环境科学与工程前沿（英文）》 2023年 第17卷 第11期 doi: 10.1007/s11783-023-1734-9

摘要：

● Photochemical conversion of chlorobenzene (CB) on α-Fe2O3 was evaluated.

关键词： Photochemical conversion     Chlorobenzene     α-Fe2O3     PCDD/Fs     Mineral particulate    

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Health impacts of air pollution in China

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1367-1

摘要：

•Impacts of air pollution on various body systems health in China were highlighted.

关键词： Health impacts     Air pollution     China     Advances    

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Environmental pollution and DNA methylation: carcinogenesis, clinical significance, and practical applications

null

《医学前沿（英文）》 2015年 第9卷 第3期   页码 261-274 doi: 10.1007/s11684-015-0406-y

摘要：

Environmental pollution is one of the main causes of human cancer. Exposures to environmental carcinogens result in genetic and epigenetic alterations which induce cell transformation. Epigenetic changes caused by environmental pollution play important roles in the development and progression of environmental pollution-related cancers. Studies on DNA methylation are among the earliest and most conducted epigenetic research linked to cancer. In this review, the roles of DNA methylation in carcinogenesis and their significance in clinical medicine were summarized, and the effects of environmental pollutants, particularly air pollutants, on DNA methylation were introduced. Furthermore, prospective applications of DNA methylation to environmental pollution detection and cancer prevention were discussed.

关键词： environmental pollution     DNA methylation     cancer     biomarker     diagnosis     therapy     prevention    

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Investigating the impact of air pollution on AMI and COPD hospital admissions in the coastal city of

《环境科学与工程前沿（英文）》 2022年 第16卷 第5期 doi: 10.1007/s11783-021-1490-7

摘要：

• The impact of air pollution on AMI/COPD hospital admissions were examined.

关键词： AMI     COPD     Air pollution exposure     GAM    

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Experimental study of pollution effect on the behavior of high voltage insulators under alternative current

Hani BENGUESMIA, Nassima M’ZIOU, Ahmed BOUBAKEUR

《能源前沿（英文）》 2021年 第15卷 第1期   页码 213-221 doi: 10.1007/s11708-017-0479-1

摘要： In this paper, the impact of the conductivity and the distribution of pollution on the behavior of the high voltage insulator cap and pin 1512L, artificially polluted is described. An experimental model in form of a disc is proposed. This experimental model reproduces the real model which is the 1512L insulator. Besides, a comparative study is presented. For this comparative study, different solutions are adopted to s`imulate the pollution (containing NaCl+ distilled water) that has different conductivities for a discontinuous distribution of the pollution on the insulator under an AC voltage. Furthermore, the influence of the pollution on the flashover voltage and the leakage current is studied. Finally, the behavior of real and experimental model of the insulator is investigated.

关键词： 1512L insulator     circular model     artificial pollution     flashover     leakage current     discontinuous pollution     high voltage    

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A critical review of the emerging research on the detection and assessment of microplastics pollution

《环境科学与工程前沿（英文）》 2022年 第16卷 第10期 doi: 10.1007/s11783-022-1563-2

摘要：

● Coastal and marine regions are the most studied for microplastic pollution.

关键词： Plastic pollution     Waste management     Global south     Sustainability     Marine pollution    

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System engineering for water pollution control at the watershed level in China

Wei MENG,

《环境科学与工程前沿（英文）》 2009年 第3卷 第4期   页码 443-452 doi: 10.1007/s11783-009-0037-0

摘要： The present water pollution situation at watershed level in China has been systematically analyzed. The causes of water pollution are attributed to the extensive economic developmental pattern, poor wastewater treatment, and a lack of nonpoint pollution control. The problems of water pollution control at watershed level include a lack of thought and approach, developmental delay in the environmental standard system, an inadequate monitoring ability, and an inefficient implementation of laws and regulations. From 2006 to 2020, water pollution control and governance will be a national key specific project of science and technology in China. The strategies of this project include establishing a water pollution control system at watershed level, orienting a healthy aquatic ecosystem, conducting risk management, and using comprehensive methods. The goal is to establish and complete a technological system of pollution control and management in three five-year phases. The main tasks are to develop common technologies, management systems, and mechanisms for lake eutrophication control, river pollution control, urban water environmental pollution control, potable water safety, and water environmental management. The bottlenecks of water pollution control and management in China could be systematically removed, and the demonstration of the system engineering approach will be conducted at selected key watersheds.

关键词： water pollution control     watershed     system engineering     sustainability     integrated watershed management     key specific project of science and technology    

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ENHANCING RAINFALL-RUNOFF POLLUTION MODELING BY INCORPORATION OF NEGLECTED PHYSICAL PROCESSES

《农业科学与工程前沿（英文）》 2023年 第10卷 第4期   页码 553-565 doi: 10.15302/J-FASE-2023519

摘要：

The growing need to mitigate rainfall-runoff pollution, especially first flush, calls for accurate quantification of pollution load and the refined understanding of its spatial-temporal variation. The wash-off model has advantages in modeling rainfall-runoff pollution due to the inclusion of two key physical processes, build-up and wash-off. However, this disregards pollution load from wet precipitation and the relationship between rainfall and runoff, leading to uncertainties in model outputs. This study integrated the Soil Conservation Service curve number (SCS-CN) into the wash-off model and added pollutant load from wet precipitation to enhance the rainfall-runoff pollution modeling. The enhanced wash-off model was validated in a typical rural-residential area. The results showed that the model performed better than the established wash-off model and the commonly-used event mean concentrations method, and identified two different modes of pollution characteristics dominated by land pollution and rainfall pollution, respectively. In addition, the model simulated more accurate pollutant concentrations at high-temporal-resolution. From this, it was found that 12% of the total runoff contained 80% to 95% of the total load for chemical oxygen demand, total N, and total P, whereas it contained only 15% of the total load for NH4+-N. The enhanced model can provide deeper insights into non-point pollution mitigation.

关键词： Erhai Lake     field experiment     non-point source     pollution load     rainfall runoff     wash-off model    

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IMPROVING NITROGEN SAFETY IN CHINA: NITROGEN FLOWS, POLLUTION AND CONTROL

《农业科学与工程前沿（英文）》 2022年 第9卷 第3期   页码 465-474 doi: 10.15302/J-FASE-2022454

摘要：

● It is necessary to address the N flows and their impacts on environment in China for sustainable N management.

关键词： barriers     future management     ammonia emissions     nitrogen input     water N pollution    

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Bacteriophages in water pollution control: Advantages and limitations

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1378-y

摘要：

•Phages can be better indicators of enteric viruses than fecal indicator bacteria.

关键词： Phage     Water pollution monitoring     Harmful bacteria biocontrol     Horizontal gene transfer     Bacterial resistance    

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Microplastics pollution and reduction strategies

Wei-Min Wu,Jun Yang,Craig S. Criddle

《环境科学与工程前沿（英文）》 2017年 第11卷 第1期 doi: 10.1007/s11783-017-0897-7

摘要： Microplastic particles smaller than 5 mm in size are of increasing concern, especially in aquatic environments, such as the ocean. Primary source is microbeads (<1 mm) used in cosmetics and cleaning agents and fiber fragments from washing of clothes, and secondary source such as broken down plastic litter and debris. These particles are mostly made from polyethylene (PE), polypropylene (PP), polystyrene (PS), polyethylene terephthalate (PET) and polyesters. They are ingested by diverse marine fauna, including zooplanktons, mussel, oyster, shrimp, fish etc. and can enter human food chains via several pathways. Strategy for control of microplastics pollution should primarily focus on source reduction and subsequently on the development of cost-effective clean up and remediation technologies. Recent research results on biodegradation of plastics have revealed a potential for microbial biodegradation and bioremediation of plastic pollutants, such as PE, PS and PET under appropriate conditions.

关键词： microplastics     plastic microbeads     environmental pollution     biodegradation    

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标题 作者 时间 类型 操作

Surface modification of biomaterials by photochemical immobilization and photograft polymerization to

Yakai FENG, Haiyang ZHAO, Li ZHANG, Jintang GUO,

期刊论文

Identification of sources, characteristics and photochemical transformations of dissolved organic matter

期刊论文

Peroxyacetyl nitrate measurements by thermal dissociation–chemical ionization mass spectrometry in an urban environment: performance and characterizations

Xinfeng Wang, Tao Wang, Likun Xue, Wei Nie, Zheng Xu, Steven C. N. Poon, Wenxing Wang

期刊论文

Photochemical indicators of ozone sensitivity: application in the Pearl River Delta, China

Lyumeng Ye,Xuemei Wang,Shaofeng Fan,Weihua Chen,Ming Chang,Shengzhen Zhou,Zhiyong Wu,Qi Fan

期刊论文

Atmospheric heterogeneous reaction of chlorobenzene on mineral -FeO particulates: a chamber experiment study

期刊论文

Health impacts of air pollution in China

期刊论文

Environmental pollution and DNA methylation: carcinogenesis, clinical significance, and practical applications

null

期刊论文

Investigating the impact of air pollution on AMI and COPD hospital admissions in the coastal city of

期刊论文

Experimental study of pollution effect on the behavior of high voltage insulators under alternative current

Hani BENGUESMIA, Nassima M’ZIOU, Ahmed BOUBAKEUR

期刊论文

A critical review of the emerging research on the detection and assessment of microplastics pollution

期刊论文

System engineering for water pollution control at the watershed level in China

Wei MENG,

期刊论文

ENHANCING RAINFALL-RUNOFF POLLUTION MODELING BY INCORPORATION OF NEGLECTED PHYSICAL PROCESSES

期刊论文

IMPROVING NITROGEN SAFETY IN CHINA: NITROGEN FLOWS, POLLUTION AND CONTROL

期刊论文

Bacteriophages in water pollution control: Advantages and limitations

期刊论文

Microplastics pollution and reduction strategies

Wei-Min Wu,Jun Yang,Craig S. Criddle

期刊论文